Atmos. Chem. Phys. Discuss., 12, 12203-12227, 2012
www.atmos-chem-phys-discuss.net/12/12203/2012/
doi:10.5194/acpd-12-12203-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Seasonal changes in gaseous elemental mercury in relation to monsoon cycling over the Northern South China Sea
C. M. Tseng1, C. S. Liu1, and C. Lamborg2
1Inst. of Oceanography, National Taiwan University, P.O. Box 23-13, Taipei 106, Taiwan
2Woods Hole Oceanographic Institute, MS 51, Woods Hole, MA 02543, USA

Abstract. The distribution of gaseous elemental mercury (GEM) was determined in the surface atmosphere of the Northern South China Sea (SCS) during 12 SEATS cruises between May 2003 and December 2005. The sampling and analysis of GEM were performed on board ship by using an on-line mercury analyzer (GEMA). Distinct annual patterns were observed for the GEM with a winter maximum of 5.7 ± 0.2 ng m−3 (n = 3) and low in summer (2.8 ± 0.2) (n = 3), with concentrations elevated 2 ∼ 3 times global background values. Source tracking through backward trajectory analysis demonstrated air masses during the northeast monsoon in winter came from Eurasia, bringing continental- and industrial-derived GEM to the SCS. In contrast, during summer southwest monsoon and inter-monsoon, air masses were from the Indochina peninsula and Indian Ocean and West Pacific Ocean. This demonstrates the impact that long-range transport, as controlled by seasonal monsoons, has on the Hg atmospheric distribution and cycling in the SCS.

Citation: Tseng, C. M., Liu, C. S., and Lamborg, C.: Seasonal changes in gaseous elemental mercury in relation to monsoon cycling over the Northern South China Sea, Atmos. Chem. Phys. Discuss., 12, 12203-12227, doi:10.5194/acpd-12-12203-2012, 2012.
 
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