Atmos. Chem. Phys. Discuss., 11, 6737-6770, 2011
www.atmos-chem-phys-discuss.net/11/6737/2011/
doi:10.5194/acpd-11-6737-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Cloud condensation nuclei as a modulator of ice processes in Arctic mixed-phase clouds
S. Lance1,2, M. D. Shupe2,3, G. Feingold1, C. A. Brock1, J. Cozic1,2, J. S. Holloway1,2, R. H. Moore4, A. Nenes4,5, J. P. Schwarz1,2, J. R. Spackman1,2, K. D. Froyd1,2, D. M. Murphy1, J. Brioude1,2, O. R. Cooper1,2, A. Stohl6, and J. F. Burkhart6,7
1Chemical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
2Cooperative Institute for Research in Environmental Sciences, University of Colorado, Boulder, CO, USA
3Physical Sciences Division, Earth System Research Laboratory, National Oceanic and Atmospheric Administration, Boulder, CO, USA
4School of Chemical & Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA
5School of Earth and Atmospheric Sciences, Georgia Institute of Technology, Atlanta, GA, USA
6Norwegian Institute for Air Research, Kjeller, Norway
7Sierra Nevada Research Institute, University of California, Merced, CA, USA

Abstract. We propose that cloud condensation nuclei (CCN) concentrations are important for modulating ice formation of Arctic mixed-phase clouds, through modification of the droplet size distribution. Aircraft observations from the Aerosol, Radiation, and Cloud Processes affecting Arctic Climate (ARCPAC) study in northern Alaska in April 2008 allow for identification and characterization of both aerosol and trace gas pollutants, which are then compared with cloud microphysical properties. Consistent with previous studies, we find that the concentration of precipitating ice particles (>400 μm) is correlated with the concentration of large droplets (>30 μm). We are further able to link the observed microphysical conditions to aerosol pollution, originating mainly from long range transport of biomass burning emissions. The case studies demonstrate that polluted mixed-phase clouds have narrower droplet size distributions and contain 1–2 orders of magnitude fewer precipitating ice particles than clean clouds at the same temperature. This suggests an aerosol indirect effect leading to greater cloud lifetime, greater cloud emissivity, and reduced precipitation. This result is opposite to the glaciation indirect effect, whereby polluted clouds are expected to precipitate more readily due to an increase in the concentration of particles acting as IN.

Citation: Lance, S., Shupe, M. D., Feingold, G., Brock, C. A., Cozic, J., Holloway, J. S., Moore, R. H., Nenes, A., Schwarz, J. P., Spackman, J. R., Froyd, K. D., Murphy, D. M., Brioude, J., Cooper, O. R., Stohl, A., and Burkhart, J. F.: Cloud condensation nuclei as a modulator of ice processes in Arctic mixed-phase clouds, Atmos. Chem. Phys. Discuss., 11, 6737-6770, doi:10.5194/acpd-11-6737-2011, 2011.
 
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