Atmos. Chem. Phys. Discuss., 11, 5379-5405, 2011
www.atmos-chem-phys-discuss.net/11/5379/2011/
doi:10.5194/acpd-11-5379-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Carbon balance of South Asia constrained by passenger aircraft CO2 measurements
P. K. Patra1, Y. Niwa2, T. J. Schuck3, C. A. M. Brenninkmeijer3, T. Machida4, H. Matsueda2, and Y. Sawa2
1Research Institute for Global Change, JAMSTEC, Yokohama 236 001, Japan
2Meteorological Research Institute, Tsukuba, Ibaraki, 305-0052 Japan
3Max Planck Institute for Chemistry, 55128 Mainz, Germany
4National Institute for Environmental Studies, Tsukuba, Ibaraki, 305-0052 Japan

Abstract. Quantifying the fluxes of carbon dioxide (CO2) between the atmosphere and terrestrial ecosystems in all their diversity, across the continents, is important and urgent for implementing effective mitigating policies. Whereas much is known for Europe and North America for instance, in comparison, South Asia, with 1.6 billion inhabitants and considerable CO2 fluxes, remained terra incognita in this respect. We use regional measurements of atmospheric CO2 aboard a Lufthansa passenger aircraft between Frankfurt (Germany) and Chennai (India) at cruise altitude, in addition to the existing network sites for 2008, to estimate monthly fluxes for 64-regions using Bayesian inversion and transport model simulations. The applicability of the model's transport parameterization is confirmed using SF6, CH4 and N2O simulations for the CARIBIC datasets. The annual carbon flux obtained by including the aircraft data is twice as large as the fluxes simulated by a terrestrial ecosystem model that was applied to prescribe the fluxes used in the inversions. It is shown that South Asia sequestered carbon at a rate of 0.37±0.20 Pg C yr−1 (1Pg C = 1015 g of carbon in CO2) for the years 2007 and 2008. The seasonality and the strength of the calculated monthly fluxes are successfully validated using independent measurements of vertical CO2 profiles over Delhi and spatial variations at cruising altitude over Asia aboard Japan Airlines passenger aircraft.

Citation: Patra, P. K., Niwa, Y., Schuck, T. J., Brenninkmeijer, C. A. M., Machida, T., Matsueda, H., and Sawa, Y.: Carbon balance of South Asia constrained by passenger aircraft CO2 measurements, Atmos. Chem. Phys. Discuss., 11, 5379-5405, doi:10.5194/acpd-11-5379-2011, 2011.
 
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