Atmos. Chem. Phys. Discuss., 11, 31851-31909, 2011
www.atmos-chem-phys-discuss.net/11/31851/2011/
doi:10.5194/acpd-11-31851-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Hindcast experiments of tropospheric composition during the summer 2010 fires over Western Russia
V. Huijnen1, J. Flemming2, J. W. Kaiser2, A. Inness2, J. Leitão3, A. Heil4, H. J. Eskes1, M. G. Schultz4, A. Benedetti2, G. Dufour5, and M. Eremenko5
1Royal Netherlands Meteorological Institute, De Bilt, The Netherlands
2European Centre for Medium-Range Weather Forecasts (ECMWF), Reading, UK
3Institute of Environmental Physics, University of Bremen, Bremen, Germany
4Forschungszentrum Jülich, Jülich, Germany
5Laboratoire Inter-universitaire des Systèmes Atmosphériques (LISA), UMR7583, CNRS/INSU – Universités Paris Est Créteil et Paris Diderot, Créteil, France

Abstract. The severe wildfires in Western Russia during July–August 2010 coincided with a strong heat wave and led to large emissions of aerosols and trace gases such as carbon monoxide (CO), hydrocarbons and nitrogen oxides into the troposphere. This extreme event is used to evaluate the ability of the global MACC (Monitoring Atmospheric Composition and Climate) atmospheric composition forecasting system to analyze large-scale pollution episodes and to test the respective influence of a priori emission information and data assimilation on the results. Daily 4-day hindcasts were conducted using assimilated aerosol optical depth (AOD), CO, nitrogen dioxide (NO2) and ozone (O3) data from a range of satellite instruments. Daily fire emissions were used from the Global Fire Assimilation System (GFAS) version 1.0, derived from satellite fire radiative power retrievals.

The impact of accurate wildfire emissions is dominant on the composition in the boundary layer, whereas the assimilation system influences concentrations throughout the troposphere, reflecting the vertical sensitivity of the satellite instruments. The application of the daily fire emissions reduces the area-average mean bias by 63% (for CO), 38% (O3) and 64% (NO2) during the first 24 h, compared to a reference simulation with a multi-annual mean climatology of biomass burning emissions. When initial tracer concentrations are further constrained by data assimilation, biases are reduced by 87, 38 and 80%. The forecast accuracy, quantified by the mean bias up to 96 h lead time, was best for all compounds when using both the GFAS emissions and assimilation. The model simulations suggest an indirect positive impact of O3 and CO assimilation on hindcasts of NO2 via changes in the oxidizing capacity.

However, the quality of local hindcasts was strongly depending on the assumptions made for forecasted fire emissions. This was well visible from a relatively rapid increase by the root mean square error with respect to ground-based data for AOD, and satellite based NO2. This calls for a more advanced method to forecast fire emissions than the currently adopted persistency approach.

The combined analysis of fire radiative power observations, multiple trace gas and aerosol satellite observations, as provided by the MACC system, results in a detailed quantitative description of the impact of major fires on atmospheric composition, and demonstrate the capabilities for the real-time analysis and forecasts of large-scale fire events.


Citation: Huijnen, V., Flemming, J., Kaiser, J. W., Inness, A., Leitão, J., Heil, A., Eskes, H. J., Schultz, M. G., Benedetti, A., Dufour, G., and Eremenko, M.: Hindcast experiments of tropospheric composition during the summer 2010 fires over Western Russia, Atmos. Chem. Phys. Discuss., 11, 31851-31909, doi:10.5194/acpd-11-31851-2011, 2011.
 
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