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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACPD</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics Discussions</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACPD</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7375</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>GÃ¶ttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acpd-11-30797-2011</article-id>
<title-group>
<article-title>Ice formation and development in aged, wintertime cumulus over the UK : observations and modelling</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Crawford</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Bower</surname>
<given-names>K. N.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Choularton</surname>
<given-names>T. W.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dearden</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Crosier</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Westbrook</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Capes</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Coe</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Connolly</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dorsey</surname>
<given-names>J. R.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gallagher</surname>
<given-names>M. W.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Williams</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Trembath</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Cui</surname>
<given-names>Z.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Blyth</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Centre for Atmospheric Science, SEAES, University of Manchester, UK</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>National Centre for Atmospheric Science, UK</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Department of Meteorology, University of Reading, UK</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Facility for Airborne Atmospheric Measurements, Cranfield University, UK</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>School of Earth and Environment, University of Leeds, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>16</day>
<month>11</month>
<year>2011</year>
</pub-date>
<volume>11</volume>
<issue>11</issue>
<fpage>30797</fpage>
<lpage>30851</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys-discuss.net/11/30797/2011/acpd-11-30797-2011.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys-discuss.net/11/30797/2011/acpd-11-30797-2011.pdf</self-uri>
<abstract>
<p>In-situ high resolution aircraft measurements of cloud microphysical
properties were made in coordination with ground based remote sensing
observations of Radar and Lidar as part of the Aerosol Properties, PRocesses
And InfluenceS on the Earth&apos;s climate (APPRAISE) project. A narrow but
extensive line (~100 km long) of shallow convective clouds over the
southern UK was studied. Cloud top temperatures were observed to be higher
than ~&amp;minus;8 Â°C, but the clouds were seen to consist of supercooled
droplets and varying concentrations of ice particles. No ice particles were
observed to be falling into the cloud tops from above. Current
parameterisations of ice nuclei (IN) numbers predict too few particles will
be active as ice nuclei to account for ice particle concentrations at the
observed near cloud top temperatures (~&amp;minus;7 Â°C). The role of
biological particles, consistent with concentrations observed near the
surface, acting as potential efficient high temperature IN is considered
important in this case. It was found that very high concentrations of ice
particles (up to 100 L&lt;sup&gt;âˆ’1&lt;/sup&gt;) could be produced by powerful secondary ice
particle production emphasising the importance of understanding primary ice
formation in slightly supercooled clouds.
&lt;br&gt;&lt;br&gt;
Aircraft penetrations at âˆ’3.5 Â°C, showed peak ice crystal
concentrations of up to 100 L&lt;sup&gt;âˆ’1&lt;/sup&gt; which together with the characteristic
ice crystal habits observed (generally rimed ice particles and columns)
suggested secondary ice production had occurred. To investigate whether the
Hallett-Mossop (HM) secondary ice production process could account for these
observations, ice splinter production rates were calculated. These calculated
rates and observations could only be reconciled provided the constraint that
only droplets &gt;24 Î¼m in diameter could lead to splinter
production, was relaxed slightly by 2 Î¼m.

&lt;br&gt;&lt;br&gt;
Model simulations of the case study were also performed with the WRF
(Weather, Research and Forecasting) model and ACPIM (Aerosol Cloud and
Precipitation Interactions Model) to investigate the likely origins of the
ice phase in these slightly supercooled clouds and to assess the role played
by the HM process in this and in controlling precipitation formation under
these conditions.
&lt;br&gt;&lt;br&gt;

WRF results showed that while HM does act to increase the mass and number
concentration of ice particles produced in the model simulations, in the
absence of HM, the ice number concentration arising from primary ice
nucleation alone (several L&lt;sup&gt;âˆ’1&lt;/sup&gt;) was apparently sufficient to sustain
precipitation although the distribution of the precipitation was changed.
Thus in the WRF model the HM process was shown to be non-critical for the
formation of precipitation in this particular case. However, this result is
seen to be subject to an important caveat concerning the simulation of the
cloud macrostructure. The model was unable to capture a sharp temperature
inversion seen in the radiosonde profiles at 2 km, and consequently the
cloud top temperature in the model was able to reach lower values than
observed in-situ or obtained from satellite data. ACPIM simulations confirmed
the HM process to be a very powerful mechanism for producing the observed
high ice concentrations, provided that primary nucleation occured to initiate
the ice formation, and large droplets were present which then fell collecting
the primary ice particles to form instant rimer particles. However, the time
to generate the observed peak ice concentrations was found to be dependant on
the number of primary IN present (decreasing with increasing IN number). This
became realistic (around 20 min) only when the temperature input to the
existing IN parameterisation was 6 Â°C lower than observed at cloud
top, highlighting the requirement to improve basic knowledge of the number
and type of IN active at these high temperatures. In simulations where cloud
droplet numbers were realistic the precipitation rate was found to be
unaffected by HM, with warm rain processes dominating precipitation
development in this instance.</p>
</abstract>
<counts><page-count count="55"/></counts>
</article-meta>
</front>
<body/>
<back>
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