Atmos. Chem. Phys. Discuss., 11, 27967-28011, 2011
www.atmos-chem-phys-discuss.net/11/27967/2011/
doi:10.5194/acpd-11-27967-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
A new real-time Lagrangian diagnostic system for stratosphere-troposphere exchange: evaluation during a balloon sonde campaign in eastern Canada
M. S. Bourqui1, A. Yamamoto1, D. Tarasick2, M. D. Moran2, L.-P. Beaudoin4, I. Beres2, J. Davies2, A. Elford2, W. Hocking3, M. Osman3, and R. Wilkinson4
1Department of Atmospheric and Oceanic Sciences, Department of Chemistry, McGill University, Montréal, Québec, Canada
2Air Quality Research Division, Environment Canada, Downsview, Ontario, Canada
3Department of Physics and Astronomy, University of Western Ontario, London, Ontario, Canada
4Canadian Space Agency, St. Hubert, Québec, Canada

Abstract. A new real-time Lagrangian diagnostic system for stratosphere-troposphere exchange (STE) developed for Environment Canada (EC) has been delivering daily archived data since 20 July 2010. The STE calculations are performed globally following the Lagrangian approach proposed in Bourqui (2006) using medium-range, high-resolution operational global weather forecasts. Following every weather forecast, trajectories are started from a dense three-dimensional grid covering the globe, and are calculated for six days of the forecast. All trajectories crossing either the dynamical tropopause (±2 PVU) or the 380 K isentrope and having a residence time greater than 12 h are archived, and also used to calculate several diagnostics. This system provides daily global STE forecasts that can be used to guide field campaigns, among other applications. The archived data set offers unique high-resolution information on transport across the tropopause for both extra-tropical hemispheres and the tropics. This will be useful for improving our understanding of STE globally, and as a reference for the evaluation of lower-resolution models. This new data set is evaluated here against measurements taken during a balloon sonde campaign with daily launches from three stations in eastern Canada (Montreal, Egbert, and Walsingham) for the period from 12 July to 4 August 2010. The campaign found an unexpectedly high number of observed stratospheric intrusions: 79% (38%) of the profiles appear to show the presence of stratospheric air below 500 hPa (700 hPa). An objective identification algorithm developed for this study is used to identify layers in the balloon-sonde profiles affected by stratospheric air and to evaluate the Lagrangian STE forecasts. We find that the predictive skill for the overall intrusion depth is excellent for intrusions penetrating down to 300 and 500 hPa, while it becomes negligible for intrusions penetrating below 700 hPa. Nevertheless, the statistical representation of these deep intrusions is reasonable, with an average bias of 24%. Evaluation of the skill at representing the detailed structures of the stratospheric intrusions shows good predictive skill down to 500 hPa, reduced predictive skill between 500 and 700 hPa, and none below. A significant low statistical bias of about 30% is found in the layer between 500 to 700 hPa. However, analysis of missed events at one site, Montreal, shows that 70% of them coincide with candidate clusters of trajectories that pass through Montreal, but that are too dispersed to be detected in the close neighbourhood of the station. This allows us to expect a negligible bias throughout the troposphere in the spatially averaged STE frequency derived from this data set, for example in climatological maps of STE mass fluxes.

Citation: Bourqui, M. S., Yamamoto, A., Tarasick, D., Moran, M. D., Beaudoin, L.-P., Beres, I., Davies, J., Elford, A., Hocking, W., Osman, M., and Wilkinson, R.: A new real-time Lagrangian diagnostic system for stratosphere-troposphere exchange: evaluation during a balloon sonde campaign in eastern Canada, Atmos. Chem. Phys. Discuss., 11, 27967-28011, doi:10.5194/acpd-11-27967-2011, 2011.
 
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