Atmos. Chem. Phys. Discuss., 11, 21013-21054, 2011
www.atmos-chem-phys-discuss.net/11/21013/2011/
doi:10.5194/acpd-11-21013-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Analysis of coherent structures and atmosphere-canopy coupling strength during the CABINEX field campaign: implications for atmospheric chemistry
A. L. Steiner1, S. N. Pressley2, A. Botros3, E. Jones4, S. H. Chung2, and S. L. Edburg5
1Department of Atmospheric, Oceanic and Space Sciences, University of Michigan, Ann Arbor, MI, USA
2Department of Civil and Environmental Engineering, Washington State University, Pullman, WA, USA
3Department of Neuroscience, University of California, Los Angeles, CA, USA
4Franklin W. Olin College of Engineering, Needham, MA, USA
5Department of Geography, University of Idaho, Moscow, ID, USA

Abstract. Intermittent coherent structures can be responsible for a large fraction of the chemical exchange between the vegetation canopy and the atmosphere. Quantifying their contribution to fluxes is necessary to interpret measurements of trace gases and aerosols within and above forest canopies. The primary objective of the Community Atmosphere-Biosphere Interactions Experiment (CABINEX) field campaign (10 July 2009 to 9 August 2009) was to study the chemistry of volatile organic compounds (VOC) within and above a forest canopy. In this manuscript, we provide an analysis of coherent structures and canopy-atmosphere exchange during CABINEX to support in-canopy gradient measurements of VOC. We quantify the number and duration of coherent structure events and their percent contribution to momentum and heat fluxes with two methods: (1) quadrant-hole analysis and (2) wavelet analysis. Despite differences in the duration and number of events, both methods predict that coherent structures contribute 40–50 % to total momentum fluxes and 44–65 % to total heat fluxes during the CABINEX campaign. Contributions associated with coherent structures are slightly greater under stable rather than unstable conditions. By comparing heat fluxes within and above the canopy, we determine the degree of coupling between upper canopy and atmosphere and find that they are coupled to the majority of the campaign time period. Uncoupled canopy-atmosphere events occur in the early morning (04:00–08:00 LT) approximately 30 % of the time. This study confirms that coherent structures contribute significantly to the exchange of heat and momentum between the canopy and atmosphere at the CABINEX site, and indicates the need to include these transport processes when studying the mixing and chemical reactions of trace gases and aerosols between a forest canopy and the atmosphere.

Citation: Steiner, A. L., Pressley, S. N., Botros, A., Jones, E., Chung, S. H., and Edburg, S. L.: Analysis of coherent structures and atmosphere-canopy coupling strength during the CABINEX field campaign: implications for atmospheric chemistry, Atmos. Chem. Phys. Discuss., 11, 21013-21054, doi:10.5194/acpd-11-21013-2011, 2011.
 
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