Atmos. Chem. Phys. Discuss., 11, 15227-15253, 2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Non-linearity in DMS aerosol-cloud-climate interactions
M. A. Thomas1,3, P. Suntharalingam1, L. Pozzoli2, A. Devasthale3, S. Kloster4,5, S. Rast5, J. Feichter5, and T. M. Lenton1
1School of Environmental Sciences, University of East Anglia, Norwich, UK
2Climate Change Unit, Joint Research Center, Italy
3Swedish Meteorological and Hydrological Institute, Norrkoping, Sweden
4Cornell University, Ithaca, NY, USA
5Max-Planck-Institute for Meteorology, Hamburg, Germany

Abstract. The degree of non-linearity in DMS-cloud-climate interactions is assessed using the ECHAM5-HAMMOZ model by taking into account end-to-end aerosol chemistry-cloud microphysics link. The evaluation is made over the Southern oceans in austral summer, a region of minimal anthropogenic influence. In this study, we compare the DMS-derived changes in the aerosol and cloud microphysical properties between a baseline simulation with the ocean DMS emissions from a prescribed climatology, and a scenario where the DMS emissions are doubled. Our results show that doubling the DMS emissions in the current climate results in a non-linear response in atmospheric DMS burden and subsequently, in SO2 and H2SO4 burdens due to inadequate OH oxidation. The aerosol optical depth increases by only ~20 % in the 30° S–75° S belt in the SH summer months. This increases the vertically integrated cloud droplet number concentrations (CDNC) by 25 %. Since the vertically integrated liquid water vapor is constant in our model simulations, an increase in CDNC leads to a reduction in cloud droplet radius of 3.4 % over the Southern oceans in summer. The equivalent increase in cloud liquid water path is 10.7 %. The above changes in cloud microphysical properties result in a change in global annual mean radiatve forcing at the TOA of −1.4 W m−2. The results suggest that the DMS-cloud microphysics link is highly non-linear. This has implications for future studies investigating the DMS-cloud climate feedbacks in a warming world and for studies evaluating geoengineering options to counteract warming by modulating low level marine clouds.

Citation: Thomas, M. A., Suntharalingam, P., Pozzoli, L., Devasthale, A., Kloster, S., Rast, S., Feichter, J., and Lenton, T. M.: Non-linearity in DMS aerosol-cloud-climate interactions, Atmos. Chem. Phys. Discuss., 11, 15227-15253, doi:10.5194/acpd-11-15227-2011, 2011.
Search ACPD
Discussion Paper
Final Revised Paper