Atmos. Chem. Phys. Discuss., 11, 1429-1455, 2011
www.atmos-chem-phys-discuss.net/11/1429/2011/
doi:10.5194/acpd-11-1429-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Mesosphere-to-stratosphere descent of odd nitrogen in February–March 2009 after sudden stratospheric warming
S.-M. Salmi1,2, P. T. Verronen1, L. Thölix1, E. Kyrölä1, L. Backman1, A. Yu. Karpechko1, and A. Seppälä1,3
1Finnish Meteorological Institute, Helsinki, Finland
2Department of Physics, University of Helsinki, Helsinki, Finland
3British Antarctic Survey (NERC), Cambridge, UK

Abstract. We use the 3-D FinROSE chemistry transport model (CTM) and ACE-FTS (Atmospheric Chemistry Experiment Fourier Transform Spectrometer) observations to study the connection between atmospheric dynamics and NOx descent during early 2009 in the northern polar region. We force the model NOx at 80 km poleward of 60° N with ACE-FTS observations and then compare the model results with observations at lower altitudes. Low geomagnetic indices indicate absence of local NOx production in early 2009, which gives a good opportunity to study the effects of atmospheric transport on polar NOx. No in-situ production of NOx by energetic particle precipitation is therefore included. This is the first model study using ECMWF (The European Centre for Medium-Range Weather Forecasts) data up to 80 km and simulating the exceptional winter of 2009 with one of the strongest major sudden stratospheric warmings (SSW). The model results show a strong NOx descent in February–March 2009 from the upper mesosphere to the stratosphere after the major SSW. Both observations and model results suggest an increase of NOx to 150–200 ppb (i.e. by factor of 50) at 65 km due to the descent following the SSW. The model, however, underestimates the amount of NOx around 55 km by 40–60 ppb. The results also show that the chemical loss of NOx was insignificant i.e. NOx was mainly controlled by the dynamics. Both ACE-FTS observations and FinROSE show a decrease of ozone of 20–30% at 30–50 km after mid-February to mid-March. However, these changes are not related to the NOx descent, but are due to activation of the halogen chemistry.

Citation: Salmi, S.-M., Verronen, P. T., Thölix, L., Kyrölä, E., Backman, L., Karpechko, A. Yu., and Seppälä, A.: Mesosphere-to-stratosphere descent of odd nitrogen in February–March 2009 after sudden stratospheric warming, Atmos. Chem. Phys. Discuss., 11, 1429-1455, doi:10.5194/acpd-11-1429-2011, 2011.
 
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