Atmos. Chem. Phys. Discuss., 11, 11379-11415, 2011
www.atmos-chem-phys-discuss.net/11/11379/2011/
doi:10.5194/acpd-11-11379-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Denitrification and polar stratospheric cloud formation during the Arctic winter 2009/2010
F. Khosrawi1, J. Urban2, M. C. Pitts3, P. Voelger4, P. Achtert1, M. Kaphlanov1, D. Murtagh2, and K.-H. Fricke*,†
1MISU, Stockholm University, Stockholm, Sweden
2Department of Radio and Space Science, Chalmers University of Technology, Göteborg, Sweden
3NASA Langley Research Center, Hampton, USA
4Swedish Institute of Space Physics (IRF), Kiruna, Sweden
*formerly at: Physikalisches Institut der Universität Bonn, Bonn, Germany
deceased, 10 August 2010

Abstract. The sedimentation of HNO3 containing Polar Stratospheric Cloud (PSC) particles leads to a permanent removal of HNO3 and thus to a denitrification of the stratosphere, an effect which plays an important role in stratospheric ozone depletion. The polar vortex in the Arctic winter 2009/2010 was very cold and stable between end of December and end of January. Strong denitrification was observed in the Arctic in mid of January by the Odin Sub Millimetre Radiometer (Odin/SMR) which was the strongest denitrification that had been observed in the entire Odin/SMR measuring period (2001–2010). Lidar measurements of PSCs were performed in the area of Kiruna, Northern Sweden with the IRF (Institutet för Rymdfysik) lidar and with the Esrange lidar in January 2010. The measurements show that PSCs were present over the area of Kiruna during the entire period of observations. The formation of PSCs during the Arctic winter 2009/2010 is investigated using a microphysical box model. Box model simulations are performed along air parcel trajectories calculated six days backward according to the PSC measurements with the ground-based lidar in the Kiruna area. From the temperature history of the trajectories and the box model simulations we find two PSC regions, one over Kiruna according to the measurements made in Kiruna and one north of Scandinavia which is much colder, reaching also temperatures below Tice. Using the box model simulations along backward trajectories together with the observations of Odin/SMR, CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) and the ground-based lidar we investigate how and by which type of PSC particles the denitrification that was observed during the Arctic winter 2009/2010 was caused. From our analysis we find that due to an unusually strong synoptic cooling event in mid January, ice particle formation on NAT may be a possible mechanism that caused denitrification during the Arctic winter 2009/2010.

Citation: Khosrawi, F., Urban, J., Pitts, M. C., Voelger, P., Achtert, P., Kaphlanov, M., Murtagh, D., and Fricke, K.-H.: Denitrification and polar stratospheric cloud formation during the Arctic winter 2009/2010, Atmos. Chem. Phys. Discuss., 11, 11379-11415, doi:10.5194/acpd-11-11379-2011, 2011.
 
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