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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>10</volume_number>
		<issue_number>3</issue_number>
		<publication_year>2010</publication_year>
	</journal>
	<doi>10.5194/acpd-10-6375-2010</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/10/6375/2010/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/10/6375/2010/acpd-10-6375-2010.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/10/6375/2010/acpd-10-6375-2010.pdf</fulltext_pdf>
	<start_page>6375</start_page>
	<end_page>6446</end_page>
	<publication_date>2010-03-08</publication_date>
	<article_title content_type="html">Two-moment bulk stratiform cloud microphysics in  the GFDL AM3 GCM: description, evaluation, and sensitivity tests</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>M. Salzmann</name>
			<email>salzmann@princeton.edu</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>Y. Ming</name>
		</author>
		<author numeration="3" affiliations="2">
			<name>J.-C. Golaz</name>
		</author>
		<author numeration="4" affiliations="2">
			<name>P. A. Ginoux</name>
		</author>
		<author numeration="5" affiliations="3">
			<name>H. Morrison</name>
		</author>
		<author numeration="6" affiliations="3">
			<name>A. Gettelman</name>
		</author>
		<author numeration="7" affiliations="4">
			<name>M. KrÃ¤mer</name>
		</author>
		<author numeration="8" affiliations="2">
			<name>L. J. Donner</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Atmospheric and Oceanic Sciences Program, Princeton University, 300 Forrestal Road, Princeton, NJ 08544, USA</affiliation>
		<affiliation numeration="2" content_type="html">Geophysical Fluid Dynamics Laboratory, NOAA, P.O. Box 308, Princeton, NJ 08542, USA</affiliation>
		<affiliation numeration="3" content_type="html">National Center for Atmospheric Research, Boulder, Colorado, USA</affiliation>
		<affiliation numeration="4" content_type="html">Forschungszentrum JÃ¼lich GmbH, ICG-I, 52425 JÃ¼lich, Germany</affiliation>
	</affiliations>
	<abstract content_type="html">A new stratiform cloud scheme including a two-moment
bulk microphysics module, a cloud cover parameterization
allowing ice supersaturation, and an ice nucleation parameterization has been
implemented into the recently developed GFDL AM3 general circulation model (GCM)
as part of an effort to treat aerosol-cloud-radiation interactions more realistically.
Unlike the original scheme, the new scheme facilitates the
study of cloud-ice-aerosol interactions via influences of dust and sulfate on ice nucleation.
While liquid and cloud ice water path associated with stratiform
clouds are similar for the new and the original scheme, column
integrated droplet numbers and  global frequency distributions
(PDFs) of droplet effective radii differ significantly. This
difference is in part due to a difference in the implementation
of the Wegener-Bergeron-Findeisen (WBF) mechanism, which leads to
a larger contribution from super-cooled droplets in the original
scheme.  Clouds are more likely to be either completely glaciated
or liquid  due to the WBF mechanism in the new scheme.
Super-saturations over ice simulated with the new scheme are in
qualitative agreement with observations, and PDFs of ice numbers
and effective radii appear reasonable in the light of observations.
Especially, the temperature dependence of ice numbers qualitatively agrees
with in-situ observations.  The global average long-wave cloud forcing
decreases in comparison to the original scheme as expected when super-saturation over ice is allowed.
Anthropogenic aerosols lead to a larger decrease in short-wave absorption
(SWABS) in the new model setup, but outgoing long-wave radiation (OLR)
decreases as well, so that the net effect of including anthropogenic
aerosols on the net radiation at the top of the atmosphere (netradTOA = SWABS-OLR)
is of similar magnitude for the new and the original scheme.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Abdul-Razzak, H. and Ghan, S J.: A parameterization of aerosol activation 2. Multiple aerosol types, J. Geophys. Res., 105, 6837â€“6844, 2000. </reference>
		<reference numeration="2" content_type="text"> Ackerman, A S., Kirkpatrick, M P., Stevens, D E., and Toon, O B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014â€“1017, 2004. </reference>
		<reference numeration="3" content_type="text"> Adler, R F., Huffman, G J., Chang, A., Ferraro, R., Xie, P.-P., Janowiak, J., Rudolf, B., Schneider, U., Curtis, S., Bolvin, D., Gruber, A., Susskind, J., Arkin, P., and Nelkin, E.: The Version-2 Global Precipitation Climatology Project (GPCP) monthly precipitation analysis (1979â€“Present), Bull. Am. Meteor. Soc., 4, 1147â€“1167, 2003. </reference>
		<reference numeration="4" content_type="text"> Albrecht, B A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227â€“1230, 1989. </reference>
		<reference numeration="5" content_type="text"> Altaratz, O., Koren, I., Reisin, T., Kostinski, A., Feingold, G., Z Levin, Z., and Yin, Y.: Aerosols&apos; influence on the interplay between condensation, evaporation and rain in warm cumulus cloud, Atmos. Chem. Phys., 8, 15â€“24, 2008. </reference>
		<reference numeration="6" content_type="text"> Andreae, M O., Jones, C D., and Cox, P M.: Strong present-day aerosol cooling implies a hot future, Nature, 435, 1187â€“1190, 2005. </reference>
		<reference numeration="7" content_type="text"> Andres, R J. and Kasgnoc, A D.: A time-averaged inventory of subaerial volcanic sulfur emissions, J. Geophys. Res., 103, 25251â€“25261, 1998. </reference>
		<reference numeration="8" content_type="text"> Austin, R T., Heymsfield, A J., and Stephens, G L.: Retrieval of ice cloud microphysical parameters using the CloudSat millimeter-wave radar and temperature, J. Geophys. Res., 114, D00A23, doi:10.1029/2008JD010 049, 2009. </reference>
		<reference numeration="9" content_type="text"> Barahona, D. and Nenes, A.: Parameterization of cirrus cloud formation in large-scale models: Homogeneous nucleation, J. Geophys. Res., 113, D11211, doi:10.1029/2007JD009 355, 2008. </reference>
		<reference numeration="10" content_type="text"> Berezinskiy, N A., Stepanov, G V., and Khorguani, V G.: Altitude variation of relative ice-forming activity of natural aerosol, S. Meterol. Hydrol., 12, 86â€“89, 1986. </reference>
		<reference numeration="11" content_type="text"> Bigg, E K.: The supercooling of water, Proc. Phys. Soc. London, 66B, 688â€“694, 1953. </reference>
		<reference numeration="12" content_type="text"> Bower, K N. and Choularton, T W.: A parameterisation of the effective radius of ice free clouds for use in global climate models, Atmos. Res., 27, 305â€“339, 1992. </reference>
		<reference numeration="13" content_type="text"> Brenguier, J L., Pawlowska, H., and SchÃ¼ller, L.: Cloud microphysical and radiative properties for parameterization and satellite monitoring of the indirect effect of aerosol on climate, J. Geophys. Res., 108, 8632, doi:10.1029/2002JD002682, 2003. </reference>
		<reference numeration="14" content_type="text"> Bretherton, C S., McCaa, J R., and Grenier, H.: A new parameterization for shallow cumulus convection and its application to marine subtropical cloud-topped boundary layers. Part I: Description and 1D results, Mon. Weather Rev., 132, 864â€“882, 2004. </reference>
		<reference numeration="15" content_type="text"> Cziczo, D J., Murphy, D M., Hudson, P K., and Thomson, D S.: Single particle measurements of the chemical composition of cirrus ice residue during CRYSTAL-FACE, J. Geophys. Res., 109, D04201, doi:10.1029/2003JD004 032, 2004. </reference>
		<reference numeration="16" content_type="text"> DeMott, P J., Rogers, R C., and Kreidenweis, S M.: The susceptability of ice formation in upper tropospheric clouds to insoluble aerosol components, J. Geophys. Res., 102, 19575â€“19584, 1997. </reference>
		<reference numeration="17" content_type="text"> Diehl, K. and Wurzler, S.: Heterogeneous drop freezing in the immersion mode: Model calculations considering soluble and insoluble particles in the drops, J. Atmos. Sci., 61, 2063â€“2072, 2004. </reference>
		<reference numeration="18" content_type="text"> Donner, L J.: A cumulus parameterization including mass fluxes, vertical momentum dynamics, and mesoscale effects, J. Atmos. Sci., 50, 889â€“906, 1993. </reference>
		<reference numeration="19" content_type="text"> Donner, L J., Seman, C J., Soden, B J., Hemler, R S., Warren, J C., StrÃ¶m, J., and k N Liou: Larce-scale ice clouds in the GFDL SKYHI general circulation model, J. Geophys. Res., 102, 21745â€“21768, 1997. </reference>
		<reference numeration="20" content_type="text"> Donner, L J., Seman, C J., and Hemler, R S.: A cumulus parameterization including mass fluxes, convective vertical velocities, and mesoscale effects: Thermodynamic and hydrological aspects in a General Circulation Model, J. Clim., 14, 3444â€“3463, 2001. </reference>
		<reference numeration="21" content_type="text"> Donner, L J., Wyman, B L., Hemler, R S., Horrowitz, L W., Ming, Y., Zhao, M., Golaz, J.-C., Austin, J., Cooke, W F., Freidenreich, S R., Ginoux, P., Gordon, C T., Griffies, S., Held, I M., Hurlin, W J., Klein, S A., Langenhurst, A R., Lee, H.-C., Lin, S.-J., Maleyshev, S L., Milly, P C D., Naik, V., Pincus, R., Polshay, J J., Ramaswamy, V., Schwarzkopf, M D., Seman, C J., Shevliakova, E., Sirutis, J J., Stern, W F., Stouffer, R J., Wilson, R J., Winton, M., and Wittenberg, A T.: The dynamical core, physical parameterizations, and basic simulation characteristics of the atmospheric component of the GFDL global coupled model CM3, in preparation, J. Climate, 2010. </reference>
		<reference numeration="22" content_type="text"> Fu, Q.: An accurate parameterization of the solar radiative properties of cirrus clouds for climate models, J. Climate, 9, 2058â€“2028, 1996. </reference>
		<reference numeration="23" content_type="text"> Fu, Q. and Liou, K N.: Parameterization of the radiative properties of cirrus clouds, J. Atmos. Sci., 50, 2008â€“2025, 1993. </reference>
		<reference numeration="24" content_type="text"> Fu, Q., Krueger, S K., and Liou, K N.: Interactions of radiation and convection in simulated tropical cloud clusters, J. Atmos. Sci., 52, 1310â€“1328, 1995. </reference>
		<reference numeration="25" content_type="text"> Georgii, H W. and Kleinjung, E.: Relations between the chemical composition of atmospheric aerosol particles and the concentration of natural ice nuclei, J. Rech. Atmos., 3, 145â€“156, 1967. </reference>
		<reference numeration="26" content_type="text"> Gettelman, A., Fetzer, E J., Eldering, A., and F W, I.: The global distribution of supersaturation in the upper troposphere from the Atmospheric Infrared Sounder, J. Climate, 19, 6089â€“6103, 2006. </reference>
		<reference numeration="27" content_type="text"> Gettelman, A., Morrison, H., and Ghan, S J.: A new two-moment bulk stratiform cloud microphysics scheme in the community atmosphere model, version 3 (CAM3). Part II: Single-colunm and global results, J. Climate, 21, 3660â€“3679, 2008. </reference>
		<reference numeration="28" content_type="text"> GFDL Global Atmospheric Model Development Team: The new GFDL global atmosphere and land model AM2-LM2: Evaluation with prescribed SST simulations, J. Atmos. Chem., 17, 4641â€“4673, 2004. </reference>
		<reference numeration="29" content_type="text"> Ghan, S J., Leung, L R., Easter, R C., and Abdul-Razzak, H.: Prediction of cloud droplet number in a general circulation model, J. Geophys. Res., 102, 21777â€“21794, 1997. </reference>
		<reference numeration="30" content_type="text"> Gierens, K., Schumann, U., Helten, M., Smit, H., and Marenco, A.: A distribution law for relative humidity in the upper troposphere and lower stratosphere derived from three years of MOZAIC measurements, Annales Geophysicae, 17, 1218â€“1226, 1999. </reference>
		<reference numeration="31" content_type="text"> Golaz, J.-C., Larson, V E., and Cotton, W R.: A PDF-based model for boundary layer clouds. Part I: Method and model description, J. Atmos. Sci., 59, 3540â€“3551, 2002. </reference>
		<reference numeration="32" content_type="text"> Golaz, J.-C., Salzmann, M., Donner, L J., Ginoux, P A., Ming, Y., and N.N.: Sensitivity to upscaling assumptions of the subgrid cloud drop activation in the GFDL AM3 GCM, J. Climate, in preparation, 2010. </reference>
		<reference numeration="33" content_type="text"> Greenwald, T J., Stephens, G L., Haar, T H V., and Jackson, D L.: A physical retrieval of cloud liquid water over the global Oceans using Special Sensor Microwave/Imager (SSM/I) observations, J. Geophys. Res., 98, 18471â€“18488, 1993. </reference>
		<reference numeration="34" content_type="text"> Hansen, J., Nazarenko, L., Ruedy, R., Sato, M., Willis, J., Genio, A D., Koch, D., Lacis, A., Lo, K., Menon, S., Novakov, T., Perlwitz, J., Russell, G., Schmidt, G A., and Tausnev, N.: Earth&apos;s Energy Imbalance: Confirmation and Implications, Science, 308, 1431â€“1435, \doi10.1126/science.1110252, http://www.sciencemag.org/cgi/content/abstract/308/5727/1431, 2005. </reference>
		<reference numeration="35" content_type="text"> Haywood, J., Donner, L., Jones, A., and Golaz, J.-C.: Global indirect radiative forcing caused by aerosols: IPPC (2007) and beyond, In: Clouds in the perturbed climate system: their relationship to energy balance, atmospheric dynamics, and precipitation, edited by: Heintzenberg, J. and Charlson, R. J., MIT Press, 451­-467, 2009. </reference>
		<reference numeration="36" content_type="text"> Heymsfield, A J.: On measurements of small ice particles in clouds, Geophys. Res. Lett., 34, L23812, doi:10.1029/2007GL030 951, 2007. </reference>
		<reference numeration="37" content_type="text"> Heymsfield, A J. and Donner, L J.: A scheme for parameterizing ice-cloud water-content in general circulation models., J. Atmos. Sci., 47, 1865â€“1877, 1990. </reference>
		<reference numeration="38" content_type="text"> Hoose, C., Lohmann, U., Edin, R., and Tegen, I.: Global influence of dust mineralogical composition on heterogeneous ice nucleation in mixed-phase clouds., Environ. Res. Lett., 3, 025003, doi:10.088/1748â€“9326/3/2/025003, 2008a. </reference>
		<reference numeration="39" content_type="text"> Hoose, C., Lohmann, U., Stier, P., Verheggen, B., and Weingartner, E.: Aerosol processing in mixed-phase clouds in ECHAM5-HAM: Model description and comparison to observations, J. Geophys. Res., 113, D07210, doi:10.1029/2007JD009 251, 2008b. </reference>
		<reference numeration="40" content_type="text"> Horowitz, L W., Walters, S., Mauzerall, D L., Emmons, L K., Rasch, P J., Garnier, C., Tie, X., Lamarque, J.-F., Schultz, M G., Tyndall, G S., Orlando, J J., and Brasseur, G P.: A global simulation of tropospheric ozone and related tracers: Description and evaluation of MOZART, version 2, J. Geophys. Res., 108, 4728, doi:10.1029/2002JD002853, 2003. </reference>
		<reference numeration="41" content_type="text"> IPCC: Climate change 2007: The physical science basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Qin, D., Manning, M., Chen, Z., Marquis, M. Aceryt, K B., Tignor, M. and Miller, H L., Cambridge University Press, Cambridge, UK and New York, NY, USA, 996 pp., 2007. </reference>
		<reference numeration="42" content_type="text"> Jakob, C.: The representation of cloud cover in atmospheric general circulation models, Ph.D. thesis, Ludwig-Maximilians-UniversitÃ¤t, MÃ¼nchen, Munich, Gemany, available at http://users.monash.edu.au/~cjakob/Papers/thesis_cjakob.pdf, 2000. </reference>
		<reference numeration="43" content_type="text"> Jakob, C. and Klein, S A.: A parameterization of the effects of cloud and precipitation overlap for use in general circulation models, Q. J. Roy. Meteorol. Soc., 126, 2525â€“2544, 2000. </reference>
		<reference numeration="44" content_type="text"> Jiang, H., Xue, H., Teller, A., Feingold, G., and Levin, Z.: Aerosol effects on the lifetime of shallow cumulus, Geophys. Res. Lett., 33, L14806, doi:1029/2006GL026024, 2006. </reference>
		<reference numeration="45" content_type="text"> KÃ¤rcher, B. and StrÃ¶m, J.: The roles of dynamical variability and aerosols in cirrus cloud formation, Atmos. Chem. Phys., 3, 823â€“838, 2003. </reference>
		<reference numeration="46" content_type="text"> KÃ¤rcher, B., MÃ¶hler, O., DeMott, P J., Pechtl, S., and Yu, F.: Insights into the role of soot aerosols in cirrus cloud formation, Atmos. Chem. Phys., 7, 4207â€“4227, 2007. </reference>
		<reference numeration="47" content_type="text"> Kessler, E.: On the distribution and continuity of water substance in atmospheric circulation, in: Meteor. Monogr., No. 32, Amer. Meteor. Soc., 84 pp., 1969. </reference>
		<reference numeration="48" content_type="text"> Khairoutdinov, M. and Kogan, Y.: A new cloud physics parameterization in a large-eddy simulation model of marine stratocumulus, Mon. Weather Rev., 128, 229â€“243, 2000. </reference>
		<reference numeration="49" content_type="text"> Koop, T., Ng, H P., Molina, L T., and Molina, M J.: A new optical technique to study aerosol phase transitions: The nucleation of ice from H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt; aerosols, J. Phys. Chem., 102A, 8924â€“8931, 1998. </reference>
		<reference numeration="50" content_type="text"> Koop, T., Luo, B., Tsias, A., and Peter, T.: Water activity as the determinant for homogeneous ice nucleation in aqueous solutions, Nature, 406, 611â€“614, 2000. </reference>
		<reference numeration="51" content_type="text"> Korolev, A V.: Limitations of the Wegener-Bergeron-Findeisen mechanism in the evolution of mixed-phase clouds, J. Atmos. Sci., 64, 3372â€“3375, 2007. </reference>
		<reference numeration="52" content_type="text"> Korolev, A V., Isaac, G A., Cober, S G., Strapp, J W., and Hallett, J.: Microphysical characterization of mixed-phase clouds, Q. J. Roy. Meteorol. Soc., 129, 39â€“65, 2003. </reference>
		<reference numeration="53" content_type="text"> KrÃ¤mer, M., Schiller, C., Afchine, A., Bauer, R., Gensch, I., Mangold, A., Schlicht, S., Spelten, N., Sitnikov, N., Borrmann, S., de~Reus, M., and Spichtinger, P.: Ice supersaturations and cirrus cloud crystal numbers, Atmos. Chem. Phys., 9, 3505â€“3522, 2009. </reference>
		<reference numeration="54" content_type="text"> KristjÃ¡nsson, J E., Edwards, J M., and Mitchell, D L.: Impact of a new scheme for optical properties of ice crystals on climates of two GCMs, J. Geophys. Res., 105, 10063â€“10079, 2000. </reference>
		<reference numeration="55" content_type="text"> Lamarque, J.-F., Granier, C., Bond, T., Eyring, V., Heil, A., Kainuma, M., Lee, D., Liousse, C., Mieville, A., Riahi, K., Schultz, M., Smith, S., Stehfest, E., Stevenson, D., Thomson, A., Aardenne, J V., and Vuuren, D V.: Gridded emissions in support of IPCC AR5, IGAC Newsletter, 41, 12â€“18, 2009. </reference>
		<reference numeration="56" content_type="text"> Li, J.-L F., Waliser, D., Woods, C., Teixeira, J., Bacmeister, J., Chern, J., Shen, B W., Tompkins, A., Tao, W K., and Kohler, M.: Comparisons of satellites liquid water estimates to ECMWF and GMAO analyses, 20th century IPCC AR4 climate simulations, and GCM simulations, J. Geophys. Res., 35, L19710, doi:10.1029/2008GL035427, 2008. </reference>
		<reference numeration="57" content_type="text"> Liu, X. and Penner, J E.: Ice nucleation parameterization for global models, Meteor. Z., 14, 499â€“514, 2005. </reference>
		<reference numeration="58" content_type="text"> Liu, X., Penner, J E., Ghan, S J., and Wang, M.: Inclusion of ice microphysics in the NCAR community atmospheric model version 3 (CAM3), J. Climate, 20, 4526â€“4547, 2007. </reference>
		<reference numeration="59" content_type="text"> Liu, X., Penner, J E., and Wang, M.: Influence of anthropogenic sulfate and black carbon on upper tropospheric clouds in the NCAR CAM3 model coupled to the IMPACT global aerosol model, J. Geophys. Res., 114, D03204, doi:10.1029/2008JD010 492, 2009. </reference>
		<reference numeration="60" content_type="text"> Lock, A P., Brown, A R., Bush, M R., Martin, G M., and Smith, R N B.: A new boundary layer mixing scheme. Part I: Scheme description and single-column model tests, Mon. Weather Rev., 128, 3187â€“3199, 2000. </reference>
		<reference numeration="61" content_type="text"> Loeb, N G., Wielicki, B A., Doelling, D R., Smith, G L., Keyes, D F., Kato, S., Manalo-Smith, N., and Wong, T.: Toward Optimal Closure of the Earth&apos;s Top-of-Atmosphere Radiation Budget, J. Climate, 22, 748â€“766, 2009. </reference>
		<reference numeration="62" content_type="text"> Lohmann, U.: A glaciation indirect aerosol effect caused by soot aerosols, Geophys. Res. Lett., 29, 1052, doi:10.1029/2001GL014 357, 2002. </reference>
		<reference numeration="63" content_type="text"> Lohmann, U. and Diehl, K.: Sensitivity studies of the importance of dust ice nuclei for the indirect aerosol effect on stratiform mixed-phase clouds, J. Atmos. Sci., 63, 968â€“982, 2006. </reference>
		<reference numeration="64" content_type="text"> Lohmann, U. and Feichter, H.: Global indirect aerosol effects: A review, Atmos. Chem. Phys., 5, 715â€“737, 2005. </reference>
		<reference numeration="65" content_type="text"> Lohmann, U. and KÃ¤rcher, B.: First interactive simulations of cirrus clouds formed by heterogeneous freezing in the ECHAM general circulation model, J. Geophys. Res., 107, 4105, doi:10.1029/2001JD000767, 2007. </reference>
		<reference numeration="66" content_type="text"> Lohmann, U., KÃ¤rcher, B., and Hendricks, J.: Sensitivity studies of cirrus clouds formed by heterogeneous freezing in the ECHAM GCM, J. Geophys. Res., 109, D16204, doi:10.1029/2003JD0004443, 2004. </reference>
		<reference numeration="67" content_type="text"> Lohmann, U., Stier, P., Hoose, C., Ferrachat, S., Kloster, S., Roeckner, E., and Zhang, J.: Cloud microphysics and aerosol indirect effects in the global climate model ECHAM5-HAM, Atmos. Chem. Phys., 7, 3425â€“3446, 2007. </reference>
		<reference numeration="68" content_type="text"> Magi, B., Ginoux, P., Ming, Y., and Ramaswamy, V.: Evaluation of tropical and extratropical Southern Hemisphere African aerosol properties simulated by a climate model, J. Geophys. Res., 114, D14204, doi:10.1029/2008JD011128, 2009. </reference>
		<reference numeration="69" content_type="text"> Manton, M J. and Cotton, W R.: Formulation of approximate equations for modeling moist deep convection on the mesoscale, Atmospheric Science Paper No. 266, Colorado State University, 62 pp., 1977. </reference>
		<reference numeration="70" content_type="text"> Martin, G M., Johnson, D W., and Spice, A.: The measurement and parameterization of effective radius of droplets in warm stratocumulus clouds, J. Atmos. Sci., 51, 1823â€“1842, 1994. </reference>
		<reference numeration="71" content_type="text"> McFarquhar, G M. and Heymsfield, A J.: Microphysical characteristics of three anvils sampled during the Central Equatorial Pacific Experiment, J. Atmos. Sci., 53, 2401â€“2423, 1996. </reference>
		<reference numeration="72" content_type="text"> McFarquhar, G M., Um, J., Freer, M., Baumgardner, D., Kok, G L., and Mace, G.: Importance of small ice crystals to cirrus properties: Observations from the Tropical Warm Pool International Cloud Experiment (TWP-ICE), Geophys. Res. Lett., 34, L13803, doi:10.1029/2007GL029 865, 2007. </reference>
		<reference numeration="73" content_type="text"> Meyers, M P., DeMott, P J., and Cotton, W R.: New primary ice nucleation parameterizations in an explicit cloud model, J. Appl. Meteorol., 32, 708â€“721, 1992. </reference>
		<reference numeration="74" content_type="text"> Ming, Y., Ramaswamy, V., Donner, L J., and Phillips, V T J.: A new parameterization of cloud droplet activation applicable to general circulation models, J. Atmos. Sci., 63, 1348â€“1356, 2006. </reference>
		<reference numeration="75" content_type="text"> Ming, Y., Ramaswamy, V., Donner, L J., Phillips, V T J., Klein, S A., Ginoux, P A., and Horowitz, L W.: Modeling the interactions between aerosols and liquid water clouds with a self-consistent cloud scheme in a general circulation model, J. Atmos. Sci., 64, 1189â€“1209, 2007. </reference>
		<reference numeration="76" content_type="text"> Minikin, A., Petzold, A., StrÃ¶m, J., Krejci, R., Seifert, M., van Velthoven, P., Schlager, H., and Schumann, U.: Aircraft observations of the upper tropospheric fine particle aerosol in the Northern and Southern Hemispheres at midlatitudes, Geophys. Res. Lett., 30, 1503, doi:10.1029/2002GL016458, 2003. </reference>
		<reference numeration="77" content_type="text"> Morrison, H. and Gettelman, A.: A new two-moment bulk stratiform cloud microphysics scheme in the community atmosphere model, version 3 (CAM3). Part I: Description and numerical tests, J. Climate, 21, 3642â€“3659, 2008. </reference>
		<reference numeration="78" content_type="text"> Morrison, H. and Grabowski, W W.: A novel approach for representing ice microphysics in models: Description and tests using a kinematic framework., J. Atmos. Sci., 65, 1528â€“1548, 2007. </reference>
		<reference numeration="79" content_type="text"> Morrison, H., Curry, J A., and Khvorostyanov, V I.: A new double-moment microphysics parameterization for application in cloud and climate models. Part I: Description, J. Atmos. Sci., 62, 1665â€“1677, 2005. </reference>
		<reference numeration="80" content_type="text"> Pawlowska, H., Grabowski, W W., and Brenguier, J.-L.: Observations of the width of cloud droplet spectra in stratocumulus, Geophys. Res. Lett., 33, L19810, doi:10.1029/2006GL026 841, 2006. </reference>
		<reference numeration="81" content_type="text"> Pincus, R., Hemler, R., and Klein, S A.: Using stochastically generated subcolumns to represent cloud structure in a large-scle model, Mon. Weather Rev., 134, 3644â€“3656, 2006. </reference>
		<reference numeration="82" content_type="text"> Putman, W M. and Lin, S.-J.: Finite-volume transport on various cubed-sphere grids, J. Comput. Phys., 227, 55â€“78, 2007. </reference>
		<reference numeration="83" content_type="text"> Rayner, N A., Parker, D E., Horton, E B., Folland, C K., Alexander, L V., Rowell, D P., Kent, E C., and Kaplan, A.: Global analyses of sea surface temperature, sea ice, and night marine air temperature since the late nineteenth century, J. Geophys. Res., 108, 4407, doi:10.1029/2002JD002 670, 2003. </reference>
		<reference numeration="84" content_type="text"> Remer, L A., R, G K., R, C L., Kaufman, Y L., Tanre, D., Mattoo, S., Vanderlei Martins, J., Ichoku, C., Koren, I., Yu, H., and Holben, B N.: Global aerosol climatology from the MODIS satellite sensors, J. Geophys. Res., 113, D14S07, doi:10.1029/2007JD009661, 2008. </reference>
		<reference numeration="85" content_type="text"> Rodi, W.: Turbulence models and their application in hydraulics. A state-of-the-art review. 3rd edn, A A. Balkema, Rotterdam, The Netherlands, 1993. </reference>
		<reference numeration="86" content_type="text"> Rossow, W B. and Schiffer, R B.: Advances in understanding clouds from ISCCP, Bull. Am. Met. Soc., 80, 2261â€“2287, 1999. </reference>
		<reference numeration="87" content_type="text"> Rotstayn, L D.: A physically based scheme for the treatment of stratiform clouds and precipitation in large-scale models. I: Description and evaluation of the microphysical processes, Q. J. Roy. Meteorol. Soc., 123, 1227â€“1282, 1997. </reference>
		<reference numeration="88" content_type="text"> Rotstayn, L D., Ryan, B F., and Katzfey, J J.: A scheme for calculation of the liquid faraction in mixed phase clouds in large-scale models, Mon. Weather Rev., 128, 1070â€“1088, 2000. </reference>
		<reference numeration="89" content_type="text"> Ryan, B F.: On the global variation of precipitating layer clouds, Bull. Am. Meteor. Soc., 77, 53â€“70, 1996. </reference>
		<reference numeration="90" content_type="text"> Scott, N A., Chedin, A., Armante, R., Francis, J., Stubenrauch, C., Chaboureau, J P., Chevallier, F., Claud, C., and Cheruy, F.: Characteristics of the TOVS pathfinder Path-B dataset, Bull. Am. Meteor. Soc., 80, 2679â€“2701, 1999. </reference>
		<reference numeration="91" content_type="text"> Seifert, A. and Beheng, K D.: A double-moment parameterization for simulating autoconversion, accretion and selfcollection, Atmos. Res., 59, 265â€“281, 2001. </reference>
		<reference numeration="92" content_type="text"> Slingo, J M.: A GCM parameterization for the shortwave radiative properties of water clouds, J. Atmos. Sci., 46, 1419â€“1427, 1989. </reference>
		<reference numeration="93" content_type="text"> Soden, B J. and Held, I M.: An assessment of climate feedbacks in coupled ocean-atmosphere models, J. Climate, 19, 3354â€“3360, 2006. </reference>
		<reference numeration="94" content_type="text"> Stephens, G L., Vane, D G., Tanelli, S., Im, E., Durden, S., Rokey, M., Reinke, D., Partain, P., Mace, G G., Austin, R., L&apos;Ecuyer, T., Haynes, J., Lebsock, M., Suzuki, K., Waliser, D., Wu, D., Kay, J., Gettelman, A., Wang, Z., and Marchand, R.: CloudSat mission: Performance and early science after the first year of operation, J. Geophys. Res., 113, D00A18, doi:10.1029/2008JD009 982, 2008. </reference>
		<reference numeration="95" content_type="text"> Storelvmo, T., Kristjansson, J E., and Lohmann, U.: Aerosol influence on mixed-phase clouds in CAM-Oslo, J. Atmos. Sci., 65, 3214â€“3230, 2008. </reference>
		<reference numeration="96" content_type="text"> Susskind, J., Piraino, P., Rokke, L., Iredell, T., and Mehta, A.: Characteristics of the TOVS Pathfinder Path A dataset, Bull. Am. Meteor. Soc., 78, 1449â€“1472, 1997. </reference>
		<reference numeration="97" content_type="text"> Tiedtke, M.: Representation of clouds in large scale models, Mon. Weather Rev., 121, 3040â€“3061, 1993. </reference>
		<reference numeration="98" content_type="text"> Tompkins, A M., Gierens, K., and RÃ¤del, G.: Ice supersaturation in the ECMWF integrated forecast system, Q. J. Roy. Meteorol. Soc., 133, 53â€“63, 2007. </reference>
		<reference numeration="99" content_type="text"> Tsushima, Y., Emori, S., Ogura, T., Kimoto, M., Webb, M J., Williams, K D., Ringer, M A., Soden, B J., Li, B., and Andronova, N.: Importance of the mixed-phase cloud distribution in the control climate for assessing the response of clouds to carbon dioxide increase: a multi-model study, Clim. Dynam., 27, 113â€“116, 2006. </reference>
		<reference numeration="100" content_type="text"> Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251â€“1256, 1974. </reference>
		<reference numeration="101" content_type="text"> Waliser, D E., Li, J., Woods, C P., Austin, R T., Bacmeister, J., Chern, J., Genio, A D., Jiang, J H., Kuang, Z., Meng, H., Minnis, P., Platnick, S., Rossow, W B., Stephens, G L., Sun-Mack, S., Tao, W.-K., Tompkins, A M., Vane, D G., Walker, C., and Wu, D.: Cloud ice: A climate model challenge with signs and expectations of progress, J. Geophys. Res., 114, D00A21, doi:10.1029/2008JD010015, 2009. </reference>
		<reference numeration="102" content_type="text"> Warren, S G., Hahn, C J., London, J., Chevin, R M., and Jenne, R L.: Global distribution of total cloud cover and cloud type amounts over land, NCAR Tech. Note TN-273+STR, National Center for Atmospheric Research, Boulder, Colorado, US, 1986. </reference>
		<reference numeration="103" content_type="text"> Warren, S G., Hahn, C J., London, J., Chevin, R M., and Jenne, R L.: Global distribution of total cloud cover and cloud type amounts over ocean, NCAR Tech. Note TN-273+STR, National Center for Atmospheric Research, Boulder, Colorado, US, 1988. </reference>
		<reference numeration="104" content_type="text"> Weng, F Z. and Grody, N C.: Retrieval of cloud liquid water using the Special Sensor Microwave Imager (SSM/I), J. Geophys. Res., 99, 25535â€“25551, 1994. </reference>
		<reference numeration="105" content_type="text"> Xie, P. and Arkin, P A.: Global precipitation: A 17-year monthly analysis based on gauge observations, satellite estimates, and numerical model outputs, Bull. Am. Meteor. Soc., 78, 2539â€“2558, 1997. </reference>
		<reference numeration="106" content_type="text"> Xue, H. and Feingold, G.: Large eddy simulations of tradewind cumuli: Investigation of aerosol indirect effects, J. Atmos. Sci., 63, 1605â€“1622, 2006. </reference>
		<reference numeration="107" content_type="text"> Zhang, Y C., Rossow, W B., Lacis, A A., Oinas, V., and Mishchenko, M I.: Calculation of radiative fluxes from the surface to top of atmosphere based on ISCCP and other global data sets: Refinements of the radiative transfer model and the input data, J. Geophys. Res., 109, D19105, doi:10.1029/2003JD004457, 2004. </reference>
	</references>
</article>

