Atmos. Chem. Phys. Discuss., 10, 5911-5945, 2010
www.atmos-chem-phys-discuss.net/10/5911/2010/
doi:10.5194/acpd-10-5911-2010
© Author(s) 2010. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Simulation of aerosol optical thickness during IMPACT (May 2008, The Netherlands) with ECHAM5-HAM
G.-J. Roelofs1, H. ten Brink2, A. Kiendler-Scharr3, G. de Leeuw4,5,6, A. Mensah3, A. Minikin7, and R. Otjes2
1Institute for Marine and Atmospheric Research Utrecht (IMAU), Utrecht University, Princetonplein 5, 3584 CC Utrecht, The Netherlands
2Energy Center Netherlands (ECN), Petten, The Netherlands
3ICG-2: Troposphere, Forschungszentrum Jülich GmbH, Germany
4Business unit Environment, Health and Safety, TNO, Utrecht, The Netherlands
5Finnish Meteorological Institute, Climate Change Unit, Helsinki, Finland
6University of Helsinki, Department of Physics, Helsinki, Finland
7Deutsches Zentrum für Luft- und Raumfahrt (DLR), Oberpfaffenhofen, Germany

Abstract. In May 2008 the measurement campaign IMPACT for observation of atmospheric aerosol and cloud properties was conducted in Cabauw (The Netherlands). With a nudged version of the coupled aerosol-climate model ECHAM5-HAM we simulate aerosol and aerosol optical thickness (AOT) for the campaign period. Synoptic scale meteorology is represented realistically and simulated concentrations of aerosol sulfate and organics at the surface are generally within a factor of two from observed values. The monthly averaged AOT from the model is 0.33, about 20% larger than observed. For selected periods of the month with relatively dry and moist conditions discrepancies are approximately −30% and +15%, respectively. Discrepancies during the dry period are partly caused by inaccurate representation of boundary layer (BL) dynamics by the model affecting the simulated AOT. The model simulates too strong exchange between the BL and the free troposphere, resulting in weaker concentration gradients at the BL top than observed for aerosol and humidity, while upward mixing from the surface layers into the BL appears to be underestimated. The results indicate that beside aerosol sulfate and organics also aerosol ammonium and nitrate significantly contribute to aerosol water uptake. The relation between particle concentration and AOT is rather weak during IMPACT. The simulated day-to-day variability of AOT follows synoptic scale advection of humidity rather than particle concentration. Even for relatively dry conditions AOT appears to be strongly influenced by the diurnal cycle of RH in the lower boundary layer, further enhanced by uptake and release of nitric acid and ammonia by aerosol water.

Citation: Roelofs, G.-J., ten Brink, H., Kiendler-Scharr, A., de Leeuw, G., Mensah, A., Minikin, A., and Otjes, R.: Simulation of aerosol optical thickness during IMPACT (May 2008, The Netherlands) with ECHAM5-HAM, Atmos. Chem. Phys. Discuss., 10, 5911-5945, doi:10.5194/acpd-10-5911-2010, 2010.
 
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