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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics Discussions</journal_title>
		<journal_url>www.atmos-chem-phys-discuss.net</journal_url>
		<issn>1680-7367</issn>
		<eissn>1680-7375</eissn>
		<volume_number>10</volume_number>
		<issue_number>1</issue_number>
		<publication_year>2010</publication_year>
	</journal>
	<doi>10.5194/acpd-10-1939-2010</doi>
	<article_url>http://www.atmos-chem-phys-discuss.net/10/1939/2010/</article_url>
	<abstract_html>http://www.atmos-chem-phys-discuss.net/10/1939/2010/acpd-10-1939-2010.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys-discuss.net/10/1939/2010/acpd-10-1939-2010.pdf</fulltext_pdf>
	<start_page>1939</start_page>
	<end_page>1956</end_page>
	<publication_date>2010-01-25</publication_date>
	<article_title content_type="html">Aerosol-induced changes of convective cloud anvils produce strong climate warming</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>I. Koren</name>
			<email>ilan.koren@weizmann.ac.il</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>L. A. Remer</name>
		</author>
		<author numeration="3" affiliations="1">
			<name>O. Altaratz</name>
		</author>
		<author numeration="4" affiliations="2,3">
			<name>J. V. Martins</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>A. Davidi</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Department of Environmental Sciences, Weizmann Institute, Rehovot 76100, Israel</affiliation>
		<affiliation numeration="2" content_type="html">Laboratory for Atmospheres, NASA Goddard Space Flight Center, Greenbelt, Maryland, USA</affiliation>
		<affiliation numeration="3" content_type="html">Department of Physics and Joint Center for Earth Systems Technology, University of Maryland, Baltimore County, USA</affiliation>
	</affiliations>
	<abstract content_type="html">The effect of aerosol on clouds poses one of the largest
      uncertainties in estimating the anthropogenic contribution to
      climate change. In contrast, even small human-induced
      perturbations in cloud coverage, lifetime, height or optical
      properties can change the instantaneous radiative energy flux
      by hundreds of watts per unit area, and this forcing can be
      either warming or cooling. Clouds and aerosols form a complex
      coupled system that, unlike greenhouse gases, have relatively
      short lifetime (hours to days) and inhomogeneous
      distribution. This and the inherent complexity of cloud
      microphysics and dynamics, and the strong coupling with
      meteorology explain why the estimation of the overall effect
      of aerosol on climate is so challenging.
&lt;br&gt;&lt;br&gt;
      Here we focus on the effect of aerosol on cloud top properties
      of deep convective clouds over the tropical Atlantic. The tops
      of these vertically developed clouds consist of mostly ice and
      can reach high levels of the atmosphere, overshooting the
      lower stratosphere and reaching altitudes greater than
      16 km. We show a link between aerosol, clouds and the free
      atmosphere wind profile that can change the magnitude and sign
      of the overall climate radiative forcing.
&lt;br&gt;&lt;br&gt;
      This study demonstrates the deep link between cloud shape and
      aerosol loading and that the overall aerosol effect in regions
      of deep convective clouds might be warming. Moreover we show
      how averaging the cloud height and optical properties over
      large regions may lead to a false cooling estimation.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Albrecht,~B A.: Aerosols, cloud microphysics and fractional cloudiness, Science, 245, 1227–1230, 1989. </reference>
		<reference numeration="2" content_type="text"> Andreae, M. O., Rosenfeld, D., Artaxo, P., Costa, A. A., Frank, G. P., Longo, K. M., and Silva-Dias, M. A. F.: Smoking rain clouds over the Amazon, Science, 303, 1337–1342, 2004. </reference>
		<reference numeration="3" content_type="text"> Charlson,~R J., Ackerman,~A S., Bender,~F A.-M., Anderson,~T L., and Liu,~Z.: On the climate forcing consequences of the albedo continuum between cloudy and clear air, Tellus B, 59, 715–727, \doi10.1111/j.1600-0889.2007.00297.x, 2007. </reference>
		<reference numeration="4" content_type="text"> Chin,~M., Rood,~R B., Lin,~S.-J., Muller,~J F., and Thompson,~A M.: Atmospheric sulfur cycle in the global model GOCART: model description and global properties, J. Geophys. Res., 105(D20), 24671–24687, \doi10.1029/2000JD900384, 2000. </reference>
		<reference numeration="5" content_type="text"> Devasthale,~A., Kruger,~O., and Grassl,~H.: Change in cloud top temperatures over Europe, IEEE Geosci. Remote Sci., 2(3), 333–336, 2005. </reference>
		<reference numeration="6" content_type="text"> Fridlind, A. M., Ackerman, A. S., Jensen, E. J., Heymsfield, A. J., Poellot, M. R., Stevens, D. E., Wang, D., Miloshevich, L. M., Baumgardner, D., Lawson, R. P., Wilson, J. C., Flagan, R. C., Seinfeld, J. H., Jonsson, H. H., VanReken, T. M., Varutbangkul, V., and Rissman, T. A.: Evidence for the predominance of mid-tropospheric aerosols as subtropical anvil cloud nuclei, Science, 304(5671), 718–22, 2004. </reference>
		<reference numeration="7" content_type="text"> Heintzenberg,~J. and Charlson,~R J. (eds.): Clouds in the perturbed climate system: their relationship to energy balance, atmospheric dynamics, and precipitation, Struengmann Forum Report, vol. 2., The MIT Press, Cambridge, MA, USA, 2009. </reference>
		<reference numeration="8" content_type="text"> Jacobson,~M Z., Kaufman,~Y J., and Rudich,~Y.: Examining feedbacks of aerosols to urban climate with a~model that treats 3-D clouds with aerosol inclusions, J. Geophys. Res., 112, D24205, \doi10.1029/2007JD008922, 2007. </reference>
		<reference numeration="9" content_type="text"> Jenkins,~G S. and Pratt,~A.: Saharan dust, lightning and tropical cyclones in the eastern tropical Atlantic during NAMMA-06, Geophys. Res. Lett., 35, L12804, \doi10.1029/2008GL033979, 2008. </reference>
		<reference numeration="10" content_type="text"> Jenkins,~G S., Pratt,~A S., and Heymsfield,~A.: Possible linkages between Saharan dust and tropical cyclone rain band invigoration in the Eastern Atlantic during NAMMA-06, Geophys. Res. Lett., 35, L08815, \doi10.1029/2008GL034072, 2008. </reference>
		<reference numeration="11" content_type="text"> Lindsey,~D T. and Fromm,~M.: Evidence of the cloud lifetime effect from wildfire-induced thunderstorms, Geophys. Res. Lett., 35, L22809, \doi10.1029/2008GL035680, 2008. </reference>
		<reference numeration="12" content_type="text"> Kaufman,~Y J. and Koren,~I.: Smoke and pollution aerosol effect on cloud cover, Science, 313, 655–658, \doi10.1126/1126232, 2006. </reference>
		<reference numeration="13" content_type="text"> Khain,~A P., BenMoshe,~N., and Pokrovsky,~A.: Factors determining the impact of aerosols on surface precipitation from clouds: an attempt at classification, J. Atmos. Sci., 65, 1721–1748, 2008a. </reference>
		<reference numeration="14" content_type="text"> Khain,~A., Cohen,~N., Lynn,~B., and Pokrovsky,~A.: Possible aerosol effects on lightning activity and structure of hurricanes, J. Atmos. Sci., 65, 3652–3677, 2008b. </reference>
		<reference numeration="15" content_type="text"> King,~M D., Menzel,~W P., Kaufman,~Y J., Tanre,~D., Gao,~B.-C., Platnick,~S., Ackerman,~S A., Remer,~L A., Pincus,~R., and Hubanks,~P A.: Cloud and aerosol properties, precipitable water, and profiles of temperature and humidity from MODIS, IEEE T. Geosci. Remote, 41, 442–458, 2003. </reference>
		<reference numeration="16" content_type="text"> Koren,~I., Kaufman,~Y J., Resonfeld,~D., Remer,~L A., and Rudich,~Y.: Aerosol invigoration and restructuring of Alantic convctive clouds, Geophys. Res. Lett., 32, L14828, doi:10.1029/2005GL023187, 2005. </reference>
		<reference numeration="17" content_type="text"> Koren,~I., Remer,~L A., Kaufman,~Y J., Rudich,~Y., and Martins,~J V.: On the twilight zone between clouds and aerosols, Geophys. Res. Lett., 34, L08805, \doi10.1029/2007GL029253, 2007. </reference>
		<reference numeration="18" content_type="text"> Koren,~I., Martins,~J V., Remer,~L A., and Afargan,~H.: Smoke invigoration versus inhibition of clouds over the Amazon, Science, 321, 946–949, 2008a. </reference>
		<reference numeration="19" content_type="text"> Koren, I., Oreopoulos, L., Feingold, G., Remer, L. A., and Altaratz, O.: How small is a small cloud?, Atmos. Chem. Phys., 8, 3855–3864, 2008b. </reference>
		<reference numeration="20" content_type="text"> Koren~I., Feingold,~G., and Remer,~L.: Deep convective clouds invigoration over the Atlantic: aerosol effect, meteorology or retrieval artifacts? Atmos. Chem. Phys., submmited, 2010. </reference>
		<reference numeration="21" content_type="text"> Nakajima,~T. and King,~M D.: Determination of the optical thickness and effective particle radius of clouds from reflected solar radiation measurements. Part 1: Theory, J. Atmos. Sci., 47, 1878–1893, 1990. </reference>
		<reference numeration="22" content_type="text"> Platnick, S., King, M. D., Ackerman, S. A., Menzel, W. P., Baum, B. A., Riedi, J. C., and Frey, R. A.: The MODIS cloud products: algorithms and examples from terra, IEEE T. Geosci. Remote Sens., 41(2), 459–473, 2003. </reference>
		<reference numeration="23" content_type="text"> Remer,~L., Kleidman,~R G., Levy,~R C., Kaufman,~Y J., Tanré,~D., Mattoo,~S., Martins,~J V., Ichoku,~C., Koren,~I., Yu,~H., and Holbenet,~B N.: Global aerosol climatology from the MODIS satellite sensors, J. Geophys. Res., 113, D14S07, doi:10.1029/2007JD009661, 2008. </reference>
		<reference numeration="24" content_type="text"> Ricchiazzi,~P., Yang,~S R., Gautier,~C., and Sowle,~D.: SBDART: a~research and teaching software tool for plane-parallel radiative transfer in the Earth&apos;s atmosphere, B. Am. Meteorol. Soc., 79(10), 2101–2114, 1998. </reference>
		<reference numeration="25" content_type="text"> Rosenfeld,~D.: Suppression of rain and snow by urban and industrial air pollution, Science, 287, 1793–1796, 2000. </reference>
		<reference numeration="26" content_type="text"> Rosenfeld,~D. and Woodley,~W L.: Deep convective clouds with sustained supercooled liquid water down to &amp;minus;37.5 \degreeC, Nature, 405, 440–442, 2000. </reference>
		<reference numeration="27" content_type="text"> Twomey,~S.: The influence of pollution on the shortwave albedo of clouds, J. Atmos. Sci., 34, 1149–1152, 1977. </reference>
		<reference numeration="28" content_type="text"> Wen,~G., Marshak,~A., Cahalan,~R F., Remer,~L A., and Kleidman,~R G.: Three-dimensional aerosol-cloud radiative interaction observed in collocated MODIS and ASTER images of cumulus cloud fields, J. Geophys. Res., 112, D13204, doi:10.1029/2006JD008267, 2007. </reference>
	</references>
</article>

