Atmos. Chem. Phys. Discuss., 10, 1659-1691, 2010
www.atmos-chem-phys-discuss.net/10/1659/2010/
doi:10.5194/acpd-10-1659-2010
© Author(s) 2010. This work is distributed
under the Creative Commons Attribution 3.0 License.
Review Status
This discussion paper has been under review for the journal Atmospheric Chemistry and Physics (ACP). Please refer to the corresponding final paper in ACP.
Direct radiative effect of aerosols emitted by transport: from road, shipping and aviation
Y. Balkanski1, G. Myhre2,3, M. Gauss2,*, G. Rädel4, E. J. Highwood4, and K. P. Shine4
1Lab. des Sciences du Climat et de l'Environnement, UMR1572, IPSL, CEA-CNRS-UVSQ, Cedex, France
2Department of Geosciences, University of Oslo, Norway
3Center for International Climate and Environmental Research-Oslo (CICERO), Oslo, Norway
4Department of Meteorology, University of Reading, Reading, UK
*now at: Norwegian Meteorological Institute, Oslo, Norway

Abstract. Aerosols and their precursors are emitted abundantly by transport activities. Transportation constitutes one of the fastest growing activities and its growth is predicted to increase significantly in the future. Previous studies have estimated the aerosol direct radiative forcing from one transport sub-sector, but only one study to our knowledge estimated the range of radiative forcing from the main aerosol components (sulphate, black carbon (BC) and organic carbon) for the whole transportation sector. In this study, we compare results from two different chemical transport models and three radiation codes under different hypothesis of mixing: internal and external mixing using emission inventories for the year 2000. The main results from this study is a positive direct radiative forcing for aerosols emitted by road traffic of +20±11 mWm−2 for an externally mixed aerosol, and of +32±13 mWm−2 when BC is internally mixed . These direct radiative forcings are much higher than the previously published estimate of +3±11 mWm−2. For transport activities from shipping, the net direct aerosol radiative forcing is negative. This forcing is dominated by the contribution of the sulphate. For both an external and an internal mixture, the radiative forcing from shipping is estimated at −26±4 mWm−2. These estimates are in very good agreement with the range of a previously published one (from −46 to −13 mWm−2) but with a much narrower range. By contrast, the direct aerosol forcing from aviation is estimated to be small, and in the range −0.9 to +0.3 mWm−2.

Citation: Balkanski, Y., Myhre, G., Gauss, M., Rädel, G., Highwood, E. J., and Shine, K. P.: Direct radiative effect of aerosols emitted by transport: from road, shipping and aviation, Atmos. Chem. Phys. Discuss., 10, 1659-1691, doi:10.5194/acpd-10-1659-2010, 2010.
 
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